13–17 Sept 2021 Virtual Conference
Virtual
Europe/Vienna timezone
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Modelling interactions between kinetics of grain boundary segregation and precipitation

16 Sept 2021, 13:10
20m
Room 12

Room 12

Oral Presentation D6. Atomic scale modelling of advanced materials - Ab initio, molecular dynamics and Monte-Carlo simulations D6_Atomic scale modelling of advanced materials - Ab initio, molecular dynamics and Monte-Carlo simulations

Speaker

Dr Daniel Scheiber (Materials Center Leoben Forschung GmbH)

Description

Grain boundary (GB) segregation is a crucial factor for controlled engineering of materials properties like toughness, creep resistance, nanocrystalline stability or electrical conductivity. An important first step to tailor such properties is the knowledge of the segregation and precipitation state resulting from specific production processes including heat treatment steps. This calls for a model that connects kinetics of segregation and precipitation to evaluate the non-equilibrium distribution of alloying elements at the GB and in the grain as function of the heat treatment and microstructure.

We present a kinetic segregation model based on the Thermodynamic Extremal Principle (TEP) and its extension to precipitation. The model combines segregation energies from DFT as well as thermodynamic data with microstructure information to compute the distribution of solutes at the GB and in the bulk based on a specified heat treatment. The simulation approach is demonstrated for two different cases: In the first case, we study a Mo alloy and consider precipitation kinetics with MatCalc and subsequent segregation with the developed kinetic model. In the second case, we report on different Fe alloys, where kinetics of segregation and precipitation are treated simultaneously and we discuss the resulting competition effects between GB segregation and precipitation for different heat treatments and compositions.

Speaker Country Austria

Author

Dr Daniel Scheiber (Materials Center Leoben Forschung GmbH)

Co-authors

Dr Erwin Povoden-Karadeniz (TU Wien) Prof. F. D. Fischer (Institute of Mechanics, Montanuniversität Leoben, 8700 Leoben, Austria) Dr Jiri Svoboda (Institute of Physics of Materials, Academy of Sciences of the Czech Republic, 61662 Brno, Czech Republic.) Prof. Kozeschnik Ernst (TU Wien, Institute of Materials Science and Technology, Getreidemarkt 9, 1060 Wien, Austria) Prof. Lorenz Romaner (Materials Center Leoben)

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