13–17 Sept 2021 Virtual Conference
Virtual
Europe/Vienna timezone
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Quantum Engineering of Spin-Filtering in WS2-based Magnetic Tunnel Junctions

13 Sept 2021, 16:20
20m
Room 1

Room 1

Oral Presentation A1. 2D materials: Fundamentals, synthesis and applications A1_Functional Materials

Speaker

Mr Victor Zatko (Unité mixte de physique CNRS/Thales)

Description

Spintronics has opened a new paradigm through the use of the spin variable as the vector of information and has been largely applied from hard drives read-heads to the STT-MRAMs. While very recent, the introduction of 2D materials in Magnetic Tunnel Junctions (MTJs) has already shown some promising properties (atomic thickness control, diffusion barrier, spin filtering…)[1]. Graphene and the 2D insulator h-BN have been the first 2D materials to show strong impact on spin transport in MTJs. It was shown that strong spin filtering occurred with the creation of an insulating spin channel in metallic graphene and metallic channel in insulating h-BN[1][2]. The recent advent of the wide TMDC family of 2D semiconductors (MoS2, WS2…) opened new opportunities for further tailoring of spintronics properties.
Here, we will detail a protocol to fabricate spin valves based on CVD grown WS2, with step by step characterizations in support (Raman spectroscopy, photoluminescence, AFM measurements…) which aims at preserving interfaces spin properties by avoiding oxidations and degradations. The fabrication process is further validated by the measurements of magnetoresistance spin signals above state of the art for 2D semiconductors based MTJs. We then present experimental results on WS2 spin-filtering tunability with thickness that we discuss in light of its peculiar thickness band-structure evolution, with Density Functional Theory calculations in support. Our work opens the way to the integration of different members of the very large TMDCs family, in order to reveal their spin transport properties in MTJs[3][4].

[1] Review: Piquemal-Banci et al. J. Phys. D: Appl. Phys. 50, 203002 (2017).

[2] Piquemal-Banci et al. ACS Nano 12, 4712 (2018).

[3] Zatko et al. ACS Nano 12, 14468 (2019)

[4] Godel, Zatko et al. ACS Appl. Nano Mater. 3, 8, 7908 (2020)

Speaker Country France

Author

Mr Victor Zatko (Unité mixte de physique CNRS/Thales)

Co-authors

Dr Bernard Servet (Thales Research and Technology) Dr Bruno DLUBAK (Unité Mixte de Physique CNRS-Thales) Dr Cecilia Mattevi (Imperial College London) Dr Florian Godel (Unité Mixte de Physique CNRS/Thales) Dr Frédéric Petroff (Unité Mixte de Physique CNRS/Thales) Dr Jean-Christophe Charlier (Université Catholique de Louvain) Dr Julian Peiro (Unité Mixte de Physique CNRS/Thales/Université Paris-Saclay) Dr Marie-Blandine MARTIN (Unité Mixte de Physique CNRS/Thales) Dr Marta Galbiati (Unité Mixte de physique CNRS/Thales) Mr Mauro Och (Imperial College London) Mr Pierre Brus (Unité mixte de Physique CNRS/Thales) Prof. Pierre Seneor (Unité Mixte de Physique CNRS/Thales) Dr Regina Galceran (Unité Mixte de Physique CNRS/Thales) Dr Simon Marie-Mutien Dubois (Université Catholique de Louvain)

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